Quantum Interference Research Articles

Quantum interference in atom-exchange reactions.

Chemical reactions, where bonds break and form, are highly dynamic quantum processes. A fundamental question is whether coherence can be preserved in chemical reactions and then harnessed to generate entangled products. Here we investigated this question by studying the 2KRb → K2 + Rb2 reaction at 500 nK, focusing on the nuclear spin degrees of freedom. We prepared the initial nuclear spins in KRb in an entangled state by lowering the magnetic field to where the spin-spin interaction dominates and characterized the preserved coherence in nuclear spin wavefunction after the reaction. We observed an interference pattern that is consistent with full coherence at the end of the reaction, suggesting that entanglement prepared within the reactants could be redistributed through the atom-exchange process.

Reconfigurable water-based metamaterial with hybrid mechanism for backward-scattering reduction

A hybrid mechanism water-based metamaterial (HMWM) with polarization conversion, absorption and phase cancellation mechanisms is proposed in this paper. The absorption and polarization conversion mechanisms are integrated by combining the water layer with polarization conversion structure, and the absorption conversion rate reaches more than 90% in the dual band (4.0–4.7 GHz and 8.2–15.7 GHz). Based on the above mechanism, the phase cancellation mechanism makes use of the opposite phase between HMWM and its mirror structure for checkerboard configuration to reduce the wideband radar cross section (RCS) by 3–18 GHz, achieving wide-angle RCS reduction and polarization insensitivity. In addition, the model realizes stealth control by adjusting RCS reduction capability under different water layer conditions. The results of simulation and experiment agree well, which fully demonstrates that the HMWM has scattering suppression capability and has potential application in multifunctional metamaterial.

On-chip tunable quantum interference in a lithium niobate-on-insulator photonic integrated circuit

On-chip tunable quantum interference in a lithium niobate-on-insulator photonic integrated circuit

The Role of Spin – Orbit Coupling in the Spin Transport FM-(G/C)N-FM

The spin transport through DNA system formed by a guanine-cytosine is studied extendedly in our work. Hence, theoretical treatment is accomplished for one magnetized active region (includes base pairs and backbone) coupled to ferromagnetic leads in parallel configuration case, throughout magnetic quantum contacts (FM-(G/C)N-FM). Our treatment is based on the tight binding model to derive obvious formula for the spin dependent transmission spectrum which is employed to investigate the spin transport through DNA junction. Our calculations are accomplished in the presence of spin-orbit coupling for strong, weak and "without backbone" regimes. The role the system spin dependent factors of the transport of (G/C)N molecule are investigated in our study. These factors include the molecular length, as well as externally applied bias voltage. Variation of these factors can enhance or suppress spin transport through (G/C)N molecule (with N=10,15,20,25. The transmission spectrum results confirm that the spin transport throughout (G/C)N is originated by a coherent tunneling process between neighboring bases through the overlapping of the LUMO orbitals of the bases. The physical mechanism is raise from quantum interference combination with molecular length and the presence of spin-orbit coupling. The best functional feature for environmental effect, which may induce dephasing such as leads temperature, is investigated. The results showed that the spin-polarized transport can be effectively regulated by the molecular length of (G/C) which can exhibit efficient spin filtering and spin switching

Fabrication of planar halfmetallic ferromagnetic Josephson junctions with long range coupling

Superconducting junctions with a ferromagnet as the weak link, where triplet correlations can transport supercurrents over a substantial distance, have been of long-standing interest. In this work, we study the triplet transport in planar La0.7Sr0.3MnO3 (LSMO) nanowire Josephson junctions with NbTi superconducting contacts. By meticulous ion etching with an artificial Pt hard mask, the NbTi/LSMO bilayer is structured to form an LSMO bridge without damaging its top layer. We observe superconducting (critical) currents of the order of 109 A/m2 in a junction with a length of 1.3 μm, and distinguishing superconducting quantum interference (SQI) patterns when sweeping a magnetic field perpendicular (B⊥) to the plane of the wire or parallel (B∥) to the plane and along the wire. The observed Gaussian-shaped SQI pattern is attributed to the diffusive transport of triplet pairs in the LSMO. Our work demonstrates that combinations of oxide magnets with conventional (s-wave) alloy superconductors can be a promising new route to realizing superconducting spintronics.

Polarization-engineered photon statistics and its tomography via optomagnonic interaction.

Cavity optomagnonics has received considerable research interest in recent years, due to the coherent magnetic Brillioun light scattering in the ferromagnetic material. Here, we theoretically propose and numerically verify a feasible scheme for the full polarization tomography on photon statistics in an optomagnonic whispering-gallery-mode microresonator system in the weak-coupling regime. By performing the polarization pre- and post-selections to manipulate the polarization states of the input and output photons, we find that the rich sub- and super-Poissonian photon statistics can be selectively generated, thanks to quantum interferences. In the parameter space of phase delay, the evolution from photon bunching to antibunching indicates the change from phase to amplitude squeezing. Our obtained result has potential applications in tunable quantum polarized light sources based on the cavity optomagnonic platform in micro-nano scale. It also offers a deeper understanding for full quantum cavity optomagnonics.

Observation of Nagaoka polarons in a Fermi-Hubbard quantum simulator.

Quantum interference can deeply alter the nature of many-body phases of matter1. In the case of the Hubbard model, Nagaoka proved that introducing a single itinerant charge can transform a paramagnetic insulator into a ferromagnet through path interference2-4. However, amicroscopic observation of this kinetic magnetism induced by individually imaged dopants has been so far elusive. Here we demonstrate the emergence of Nagaoka polarons in a Hubbard system realized with strongly interacting fermions in a triangular optical lattice5,6. Using quantum gas microscopy, we image these polarons asextended ferromagnetic bubbles around particle dopants arising from the local interplay of coherent dopant motion and spin exchange. By contrast, kinetic frustration due to the triangular geometry promotes antiferromagnetic polarons around hole dopants7. Our work augurs the exploration of exotic quantum phases driven by charge motion in strongly correlated systems and over sizes that are challenging for numerical simulation8-10.

Glory interference spectroscopy in Sr atom

Slow (meV) photoelectron imaging spectroscopy is employed in the experimental study of near-threshold photoionization of strontium atoms in the presence of an external static electric field. Specifically, the study is devoted to the glory effect, that is, the appearance of an intense peak at the center of the recorded photoelectron images, when dealing with m= 0 final ionized Stark states (m denoting the magnetic quantum number). This critical effect is formally identical to that encountered in classical scattering theory, where, for a nonzero value of the impact parameter, the zero-crossing of the deflection function leads to a divergent classical differential cross section. By recording the magnitude variation of this glory peak as a function of electron excitation energy, we observe that, besides the traces of classical origin, it also exhibits intense quantum interference and beating phenomena, above and below the zero-static-field ionization threshold. We study both, single- and two-photon ionization of Sr, thus enabling a comparison not only between the different excitation schemes, but also with an earlier work devoted to two-photon ionization of Mg atom by Kalaitzis et al (2020 Phys. Rev. A 102 033101). Our recordings are analyzed within the framework of the Harmin–Fano frame transformation Stark effect theory that is applied to both the hydrogen atom and a non-hydrogenic one simulating Sr. We discuss the various aspects of the recorded and calculated glory interference and beating structures and their ‘short time Fourier transforms’ and classify them as either atom-specific or atom independent. In particular, we verify the ‘universal’ connection between the glory oscillations above the zero-field threshold and the differences between the origin-to-detector times of flight corresponding to pairs of classical electron trajectories that end up to the image center.

Influence of Severe Plastic Deformation on the Magnetic Properties of Sm–Co Permanent Magnets

High pressure torsion (HPT) is presented as a new fabrication route to produce bulk Sm–Co magnets with a strongly refined microstructure down to the nanometer regime. The initial powders, based on the compositions SmCo5, Sm2Co7 and Sm2Co17, are compacted and subsequently deformed by HPT. The microstructural evolution in dependence on the applied deformation parameters is characterized by electron microscopy and the effect of HPT on the phase stability is monitored by synchrotron X‐ray diffraction. An increasing amount of applied strain leads to a stronger reduction in grain size while strain localization counteracts a homogeneous microstructural refinement. The positive effect of elevated deformation temperatures is demonstrated for Sm2Co17, which promotes homogeneous grain refinement, but causes strain‐induced phase transformations at the same time, strongly affecting the magnetic behavior. Superconducting quantum interference device magnetometry is used to characterize the magnetic properties after HPT deformation, which indicates the formation of a magnetic texture depending on the respective phase.

Interference is in the eye of the beholder: Application to the coherent control of collisional processes.

Interference is widely regarded as a foundational attribute of quantum mechanics. However, for a given experimental arrangement, interference can either contribute or not contribute to the outcome depending upon the basis in which it is measured. This observation is both foundational and particularly relevant to coherent control of molecular processes, an approach based upon quantum interference. Here, we address this issue and its relevance to controlling molecular processes via the "coherent control scattering (CCS) matrix," a formalism that allows for an analysis of modifications in an interference structure resulting from a change of basis. This analysis reveals that the change in the interference structure can be attributed to the non-commutativity of the transformation matrix with the CCS matrix and the non-orthogonality of the transformation. Additionally, minimal interference is shown to be associated with the CCS eigenbasis and that the Fourier transform of the eigenvectors of the CCS matrix provides the maximal interference and hence the best coherent control. The change of controllability through a change of basis is illustrated with an example of 85Rb+ 85Rb scattering. In addition, the developed formalism is applied to explain recent experimental results on He + D2 inelastic scattering demonstrating the presence or absence of interference depending on the basis.

Microwave quantum memcapacitor effect

Developing the field of neuromorphic quantum computing necessitates designing scalable quantum memory devices. Here, we propose a superconducting quantum memory device in the microwave regime, termed a microwave quantum memcapacitor. It comprises two linked resonators, the primary one is coupled to a Superconducting Quantum Interference Device, which allows for the modulation of the resonator properties through external magnetic flux. The auxiliary resonator, operated through weak measurements, provides feedback to the primary resonator, ensuring stable memory behavior. This device operates with a classical input in one cavity while reading the response in the other, serving as a fundamental building block toward arrays of microwave quantum memcapacitors. We observe that a bipartite setup can retain its memory behavior and gains entanglement and quantum correlations. Our findings pave the way for the experimental implementation of memcapacitive superconducting quantum devices and memory device arrays for neuromorphic quantum computing.

Arrays of nano-high-transition temperature superconductor quantum interference devices

We report the fabrication and testing of arrays of nanoscale superconducting quantum interference devices (SQUIDs) directly written into a thin film of the high-transition temperature superconductor YBa2Cu-3O7−δ with a focused helium ion beam. We compare three array configurations with 400 nm by 400 nm nanoSQUIDs connected in series and parallel and a two-dimensional (2D) combination of both. Our electrical transport measurements show that series arrays of three nanoSQUIDs exhibit modulation voltages greater than 1 mV and that combining the devices in parallel greatly enhances the slope of the voltage–magnetic field characteristic. A 2D array with 3 SQUIDS in series and 7 in parallel exhibited a transfer function of 5.51 mV/mT.

Wideband-tunable microwave photonic filter using dissipative self-interference microring resonators

We propose and demonstrate a widely tunable microwave photonic filter with controlled frequency agility, bandwidth reconfigurability and flexible switching functions. It is based on the self-interference microring aided by an asymmetric Mach–Zehnder interferometer, breaking the fundamental microring footprint limit and achieving a doubled free spectral range (123.2 GHz) with a strong out-of-band rejection. Simulation results show that a bandpass microwave photonic filter can be tuned across a 60 GHz frequency range with a varied 3-dB bandwidth from 2.13 GHz to 40.7 GHz in a cascaded dual-ring topology. Its RF out-of-band rejection ratio is improved by more than 60 dB in the high frequency region due to a perfect residual phase cancellation. A dual-band notch microwave photonic filter with an extinction ratio of about 50 dB and a frequency tunable range of about 27.7 GHz is also demonstrated, showing its broadly applicability. Our method highlights its suitability to improve chip-scale wideband and high-performance RF receiver systems.

The SQUID Controller Unit for the LiteBIRD Space Mission: Description, Functional Tests and Early Performance Assessment

AbstractLiteBIRD is a satellite mission to be launched by JAXA in the early 2030s. It will measure the Cosmic Microwave Background (CMB) primordial B-modes with an unprecedented sensitivity. Microwave radiation will be detected by Transition Edge Sensors (TESs) arrays multiplexed in frequency domain and read by Superconducting QUantum Interference Devices (SQUIDs). The LiteBIRD SQUID Controller Unit (SCU), based on the heritage of the successful design used for the ground-based SPT3G experiment, presents some novel elements that make it suitable for a space-borne application. We compare our first breadboard model with the ground-based, Off-The-Shelf Components (COTS) version, by driving the same SQUID Array Amplifier (SAA) at 4 K, measuring relevant quantities such as noise, gain and bandwidth. We demonstrate that the noise added by our first prototype (including a switching part for redundancy purposes) never exceeds the noise added by the COTS-based electronics board, representing our benchmark. We also present the first noise estimates with the SAA cooled below 1 K, going closer to the conditions expected for LiteBIRD operation.

Photon-assisted destructive interference through a parallel-coupled double quantum dots

In this paper, we establish a model to realize the photon-assisted destructive interference phenomena, the model consisting of parallel-coupled double quantum dots and Luttinger liquid leads. By applying the canonical transformation and the nonequilibrium Green’s function technique, the general time-dependent current formula is developed. The joint effects of the intralead Coulomb interaction and an external ac field on the quantum interference are investigated. For weak intralead interactions, besides the usual photon-assisted tunneling resonance, there are two types of photon-assisted tunneling destructive interference: one is related to interdot coupling and the other to intralead interactions. For moderately strong intralead interaction, the photon-assisted sidebands are suppressed and the differential conductance scales as a power law in bias voltage. In particular, we show the multiphoton absorption and emission up to four photons in an electron tunneling process. We believe that the photo-assisted destructive interference results obtained in this paper are instructive for future experiments.

Surface plasmon induced quantum interference at meta-material interface

In this work we investigate quantum interference in a four-level atom coupled to a negative index meta-material (NIMM) anisotropic plasmonic environment that supports both TE and TM polarized surface plasmons (SP). The analysis confirms the creation of the anisotropic environment and two dipoles can interfere with each other even if they are orthogonal by sharing such SP modes. The NIMM/plasmonic environment provides more options to control SP interaction with emitters and their spontaneous emission decays and spectrum. The spectrum depends critically on structure parameters, mode frequency, frequency dependent electric permittivity and magnetic permeability, and the location of the atom etc. We observe orders of magnitudes enhancement in the plasmonic-modified decays and spectrum compared to free space case.

Estimation with Ultimate Quantum Precision of the Transverse Displacement between Two Photons via Two-Photon Interference Sampling Measurements.

We present a quantum sensing scheme achieving the ultimate quantum sensitivity in the estimation of the transverse displacement between two photons interfering at a balanced beam splitter, based on transverse-momentum sampling measurements at the output. This scheme can possibly lead to enhanced high-precision nanoscopic techniques, such as superresolved single-molecule localization microscopy with quantum dots, by circumventing the requirements in standard direct imaging of camera resolution at the diffraction limit, and of highly magnifying objectives. Interestingly, we show that our interferometric technique achieves the ultimate spatial precision in nature irrespectively of the overlap of the two displaced photonic wave packets, while its precision is only reduced of a constant factor for photons differing in any nonspatial degrees of freedom. This opens a new research paradigm based on the interface between spatially resolved quantum interference and quantum-enhanced spatial sensitivity.

Controllable quantum scars induced by spin–orbit couplings in quantum dots

Spin–orbit couplings (SOCs), originating from the relativistic corrections in the Dirac equation, offer nonlinearity in the classical limit and are capable of driving chaotic dynamics. In a nanoscale quantum dot confined by a two-dimensional parabolic potential with SOCs, various quantum scar states emerge quasi-periodically in the eigenstates of the system, when the ratio of confinement energies in the two directions is nearly commensurable. The scars, displaying both quantum interference and classical trajectory features on the electron density, due to relativistic effects, serve as a bridge between the classical and quantum behaviors of the system. When the strengths of Rashba and Dresselhaus SOCs are identical, the chaos in the classical limit is eliminated as the classical Hamilton’s equations become linear, leading to the disappearance of all quantum scar states. Importantly, the quantum scars induced by SOCs are robust against small perturbations of system parameters. With precise control achievable through external gating, the quantum scar induced by Rashba SOC is fully controllable and detectable.

Study of Molecular Dimer Morphology Based on Organic Spin Centers: Nitronyl Nitroxide Radicals.

In this work, in order to investigate the short-range interactions between molecules, the spin-magnetic unit nitronyl nitroxide (NN) was introduced to synthesize self-assembly single radical molecules with hydrogen bond donors and acceptors. The structures and magnetic properties were extensively investigated and characterized by UV-Vis absorption spectroscopy, electron paramagnetic resonance (EPR), and superconducting quantum interference devices (SQUIDs). Interestingly, it was observed that the single molecules can form two different dimers (ring-closed dimer and "L"-type dimer) in different solvents, due to hydrogen bonding, when using EPR to track the molecular spin interactions. Both dimers exhibit ferromagnetic properties (for ring-closed dimer, J/kB = 0.18 K and ΔES-T = 0.0071 kcal/mol; for "L"-type dimer, the values were J/kB = 9.26 K and ΔES-T = 0.037 kcal/mol). In addition, the morphologies of the fibers formed by the two dimers were characterized by transmission electron microscopy (TEM) and atomic force microscopy (AFM).

Effects of Connectivity Isomerization on Electron Transport Through Thiophene Heterocyclic Molecular Junction.

Connectivity isomerization of the same aromatic molecular core with different substitution positions profoundly affects electron transport pathways and single-molecule conductance. Herein, we designed and synthesized all connectivity isomers of a thiophene (TP) aromatic ring substituted by two dihydrobenzo[b]thiophene (BT) groups with ethynyl spacers (m,n-TP-BT, (m,n = 2,3; 2,4; 2,5; 3,4)), to systematically probe how connectivity contributes to single-molecule conductance. Single-molecule conductance measurements using a scanning tunneling microscopy break junction (STM-BJ) technique show ∼12-fold change in conductance values, which follow an order of 10-4.83 G0 (2,4-TP-BT) < 10-4.78 G0 (3,4-TP-BT) < 10-4.06 G0 (2,3-TP-BT) < 10-3.75 G0 (2,5-TP-BT). Electronic structure analysis and theoretical simulations show that the connectivity isomerization significantly changes electron delocalization and HOMO-LUMO energy gaps. Moreover, the connectivity-dependent molecular structures lead to different quantum interference (QI) effects in electron transport, e.g., a strong destructive QI near E = EF leads the smallest conductance value for 2,4-TP-BT. This work proves a clear relationship between the connectivity isomerization and single-molecule conductance of thiophene heterocyclic molecular junctions for the future design of molecular devices.